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A A E C / E 5 1 9

AUSTRALIAN ATOMIC ENERGY COMMISSION

RESEARCH ESTABLISHMENT LUCAS HEIGHTS

A A E C T R I T I U M LIST NO. 4 979-1980

by

G.E. C A L F R.C. S T O K E S

J u i y 198

ISBN 0 642 59715 4

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AUSTRALIAN ATOMIC ENERGY COMMISSION RESEARCH ESTABLISHMENT

LUCAS HEIGHTS

AAEC TRITIUM LIST NO. 4 1979-1980

by

G.E. CALF R.C. STOKES

ABSTRACT

Details are given of the concentration of the environmental isotope tritium in monthly precipitation samples taken at 16 stations, situated throughout Australia, during the period 1979-1980.

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National Library of Australia card number and ISBN 0 642 59715 4

The following descriptors have been selected from the INIS Thesaurus to describe the subject content of this report for information retrieval purposes. For further details please refer to IAEA-INIS-12 (INIS: Manual for Indexing) and IAEA-INIS-13 (INIS: Thesaurus) published in Vienna by the International Atomic Energy Agency.

ATMOSPHERIC PRECIPITATIONS; RADIOACTIVITY; RADIATION MONITORING; SAMPLING;

TRITIUM; AUSTRALIA

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CONTENTS

Page 1. INTRODUCTION 1 2. STATION DATA 1 3. SAMPLE ANALYSIS 1 4. RESULTS 2 5. ACKNOWLEDGEMENTS 2 6. REFERENCES 2 Table 1 Adelaide 5 Table 2 Alice Springs 6 Table 3 Brisbane 7 Table 4 Bundaberg 8 Table 5 Campbelltown 9 Table 6 Charleville 10 Table 7 Claredale 11 Table 8 Darwin 12 Table 9 Hobart 13 Table 10 Longreach 14 Table 11 Mackay 15 Table 12 Melbourne 16 Table 13 Narrabri 17 Table 14 Perth 18 Table 15 Ryde 19 Table 16 Toowoomba 20

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1.

INTRODUCTION

Since 1970, monthly precipitation samples have been collected for the

Australian Atomic Energy Commission from sixteen stations in Australia. Previous publications included data from 1970 to 1974 [Calf et al. 1976) , 1975 to 1976

[Calf et al. 1977] and 1977 to 1978 [Calf & Stokes 1979]. Precipitation survey stations are shown in Figure 1.

DARWIN

XCLAREDALE MACKAY I LONGREACH

BUNDABERG N

CHARLEVILLE

T O O W O O M B A - 4 BRISBANE

PERTH

S Y D N E Y CAMPBELLTOWN

(^—1

u

HOBART

FIGURE 1

2. STATION DATA

Basic information, including latitude, longitude and altitude are given for each location for which the tritium activity is reported.

3. SAMPLE ANALYSIS

Samples are composites from the total precipitation at a station during one calendar month and were assayed using methods reported by Calf, Seatonberry &

Smith [1975]. The tritium concentration, given in tritium units (TU), has been corrected for decay to the last day of the sampling month. One TU is defined as one atom of tritium per 10 atoms of hydrogen and is equivalent to 3.19 pCi1 fl

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(118 mBq) per litre of water if a half-life of 12.43 years is assumed. All results have an estimated standard deviation of 8.5 per cent or 0.4 TU, whichever is the larger.

4. RESULTS

Yearly weighted means for tritium, weighted by the total amount of precipitation, have been calculated according to the formula

. , , E(monthly precipitation x monthly tritium concentration) Weighted mean = — — *-=-; -r~, . . , . . :

E(monthly precipitation)

The figures in parenthesis represent the percentage of the total precipitation for which tritium data are available to calculate the weighted means.

5. ACKNOWLEDGEMENTS

We wish to acknowledge the assistance of the Department of Science & the Environment's Bureau of Meteorology, the Water Resources Commission of NSW and the Water Resources Commission of Queensland in collecting the samples and relaying the relevant monthly precipitation values.

6. REFERENCES

Calf, G.E., Seatonberry, B.W. & Smith, L.W. [1975] - The Measurement of Natural Levels of Tritium in Water. AAEC/E373.

Calf, G.E., Seatonberry, B.W., Smith, L.W. & Stokes, R.C. [1976] - AAEC Tritium List No. 1 1970-1974. AAEC/E377.

Calf, G.E., Smith, L.W. & Stokes, R.C. [1977] - AAEC Tritium List No. 2 1975-1976. AAEC/E414.

Calf, G.E. & Stokes, R.C. [1979] - AAEC Tritium List No. 3 1977-1978.

AAEC/E473.

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MONTHLY TRITIUM PRECIPITATION DATA

The following reference symbols apply to all tables in this set:

(a) Precipitation in mm.

(b) TU = tritium unit.

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TABLE 1

ADELAIDE Station : 023054

Latitude: 34 57S Longitude: 138 32 E Altitude: 7 .6 m

Year 1 1979

Month 01 02 03 04 05 06 07 08 09 10 11 12

Precipitation (?-}

29 12 11 38 54 16 46 90 101 44 37 34 Sum 512

Type rain

TU ^' 8.7 7.6 8.4 7.4 7.1 4.5 6.5 8.7 10.7 9.1 10.9 6.7

Weighted Mean 8.5 (100.0%) 1980 01

02 03 04 05 06 07 08 09 10 11 12

3 0 2 48 37 78 64 17 18 89 29 30 Sum 415

rain 11.4

7.9 6.9 7.1 4.8 4.9 4.3 9.1 9.8 6.8

Weighted Mean 7.2 (99.5%)

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ALICE SPRINGS Station : 015590

Latitude: 23 49S Longitude: 133 54E Altitude: 542.0 m

Year 1979

Month 01 02 03 04 05 06 07 08 09 10 11 12

Precipitation (a) 76

19 44 25 74 1 0 1 28

6 28

5 Sum 307

Type rain

TU (b)

7.5 11.2 6.4 6.8 6.2

11.0

8.8 6.5

Weighted Mean 7.6 (97.4%) 1980 01

02 03 04 05 06 07 08 09 10 11 12

8 7 0 26 39 7 11 5 0 44 0 22 Sum 169

rain

5.9 7.8 10.0 8.3 9.4

9.3 11.0

Weighted Mean 8.1 (78.1%)

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;LE 3

BRISBANE Station : 040223

Latitude: 27 26S Longitude: 153 05E Altitude: 2.1 m

Year 1979

Month 01 02 03 04 05 06 07 08 09 10 11 12

Precipitation (a) 167

64 52 77 8 62 40 3 1 85 98 64 Sum 721

Type i." <—L i I x

T'J (V

4.6 6.6 6.7 5.6 6.8 4.1 5.5 5.5

4.1 6.7 6.6

Weighted Mean 5.5 (99.9%) 1980 01

02 03 04 05 06 07 08 09 10 11 12

158 87 6 26 382 19 21 31 0 107

25 173

Sum 1035

rain 6.7 4.0 7.2 3.6 4.5 5.4 9.3 8.4 9.2 4.3 8.1 5.2

Weighted Mean 5.2(100.0%)

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BUNDABERG Station : 039015

Latitude: 24 52S Longitude: 152 21E Altitude: 13.7 m

Year 1979

Month 01 02 03 04 05 06 07 08 09 10 11 12

Precipitation (a) 43

76 118 35 4 26 6 4 4 69 54 38 Sum 477

Type rain

TU (*>>

5.0 3.7 4.8 4.0

3.6

10.8 5.6 4.2 7.1 3.7

Weighted Mean 4^7 (97.9%) 1980 01

02 03 04 05 06 07 08 09 10 11 12

216 242 15 18 38 37 29 12 0 81 48 107 Sum 843

rain 3.3 3.2

3.1 3.5 6.6 5.6 5.6

4.5 4.8 4.2

Weighted Mean 3.9 (98.2%)

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TABLE 5

CAMPBELLTOWN Station : 068081

Latitude: 34 07S Longitude : 150 49E Altitude: 65.0 m

Year 1979

Month 01 02 03 04 05 06 07 08 09 10 11 12

Precipitation (a) 20

10 65 39 66 55 22 3 23 43 75 4 Sum 425

Type rain

TU (b>

8.3 6.8

8.6 4.8 3.8 9.2 13.1

12.6 12.1 6.6

Weighted Mean 8.3 (79.3%) 1980 01

02 03 04 05 ' 06

07 08 9 10 11 12

85 32 27 6 116

30 20 5 0 36 41 49 Sum 448

rain 12.0 5.9 6.9 7.8 4.1 5.4 3.3 11.0

12.7 10.1 7.9

Weighted Mean 7.7 (100.0%)

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TABLE 6

CHARLEVILLE Station : 044021

Latitude: 26 25S Longitude: 146 17E Altitude: 303.9 m

Year 1979

Month 01 02 03 04 05 06 07 08 09 10 11 12

Precipitation (a) 14

82 35 18 32 21 1 4 30 20 9 6 Sum 272

Type rain

TU '^

8.1 7.7 7.6 7.0 6.5 5.4

15.3 11.2 9.0 9.3 8.8

Weighted Mean 8.0 (99.6%) 1980 01

02 03 04 05 06 07 08 09 10 11 12

43 41 39 8 25

3 44 17 0 124

18 57 Sum 419

rain 6.7 6.4 4.2 9:9 3.6

7.7 7.5

8.5 16.1 6.3

Weighted Mean 7.3 (99.3%)

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11

TABLE 7

CLAREDALE Station : 033011

Latitude: 19 35S Longitude: 147 24E Altitude: 9.7 m

Year 1979

Month 01 02 03 04 05 06 07 08 09 10 11 12

Precipitation (a) * 204

450 543 60 9 58 15 0 10 4 2 123

Sum 1478

Type rain

TU (b>

3.9 3.4 3.5 2.6

2.7 4.3

2.0 3.4 2.8

Weighted Mean 3.4 (98.7%) 1980 01

02 03 04 05 06 07 08 09 10 11 12

240 124 230 18 97 0 3 5 0 10 7 55 Sum 789

rain 2.9 3.5 2.3 2.1 2.8 6.7 4.1

2.9 2.7 3.7

Weighted Mean 2.8 (99.4%) The precipitation figures are for Ayr, which is situated 28 km from Claredale. No precipitation figures for Claredale are available.

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TABLE 8

DARWIN Station : 014015

Latitude: 12 25S Longitude: 130 52E Altitude: 28.6 m

Year 1979

Month 01 02 03 04 05 06 07 08 09 10 11 12

P "*" s c ^ T1^ "** H t i on v ^ / 444

143 228 38 64 0 0 0 3 76 37 164

Sum 1197

Type rain

TU (b>

6.3 6.4 4.2 4.1 3.6

3.5 4.8 5.4 5.5

Weighted Mean 5.5 (100.0%) 1980 01

02 03 04 05 06 07 08 09 10 11 12

694 361 236 39 0 0 0 32 0 62 159 262

Sum 1845

rain 4.1 4.1 3.2 5.4

4.5

5.1 4.9 3.3

Weighted Mean 4.0 (100.0%)

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13 TABLE 9

HOBART Station : 094029

Latitude: 42 53S Longitude: 147 20E Altitude: 55.2 m

Year 1979

Month 01 02 03 04 05 06 07 08 09 10 11 12

Precipitation (a) 39

33 27 24 19 2 12 71 66 38 18 42 Sum 391

Type rain

TU (b) 1 12.0

6.5 7.9 5.3 6.1

8.6 8.2 15.6 9.7 7.7 7.0

Weighted Mean 9.4 (99.5%) 1980 01

02 03 04 05 06 07 08 09 10 11 12

8 28 58 27 22 45 30 37 67 73 43 27 Sum 465

rain 6.9 7.8 9.2 5.8 4.3 5.6 4.3 5.0 5.4 10.9

7.5 6.0

Weighted Mean 7.0 (100.0%)

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TABLE 10 LONGREACH

Latitude: 23 26S Longitude Altitude: 190.5 m

Station : 036031 144 16E

Year 1979

Month 01 02 03 04 05 06 07 08 09 10 11 12

Precipitation (a) 15

134 62 7 5 24 0 0 8 34 2 4 Sum 295

Type rain

TU (b) 7.2 5.6 4.8 3.9 33.0 4.6

9.0 6.3 15.9

Weighted Mean 6.1 (98.6%) 1980 01

02 03 04 05 06 07 08 09 10 11 12

193 138 122 5 22 0 17

7 0 22 16 56 Sum 598

rain 4.7 7.8 5. .3 10.6

3.9

10.2 7.4

7.3 8.4 7.2

Weighted Mean 6.2 (100.0%)

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15 TABLE 11

MACKAY Station : 033119

Latitude: 21 07S Longitude: 149 13E Altitude: 30.8 m

Year 1979

Month 01 02 03 04 05 06 07 08 09 10 11 12

Precipitation (a) 587

776 584 72 47 146 62 3 4 49 36 117 Sum 2483

Type rain

TTI (b) 4.3 3.6 3.2 2.4 2.3 3.7 5.3 5.7 4.2 3.8 4.7 2.3

Weighted Mean 3.6 (100.0%) 1980 01

02 03 04 05 06 07 08 09 10 11 12

239 188 137 151 130 11 48 39 0 19 43 178

Sum 1183

rain 2.4 3.4 3.4 2.6 2.6 5.8 3.6 4.4

3.4 3.2 4.3

Weighted Mean 3.2 (100.0%)

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MELBOURNE Station : 086071

Latitude: 37 49S Longitude: 144 58E Altitude: 34.7 m

Year 1979

Month 01 02 03 04 05 06 07 08 09 10 11 12

Precipitation (a)

JO

43 27 45 89 17 9 64 62 112 27 12 Sum 543

Type rain

,-,.

~1

•ru 1~/

10. 5 9.3 11.6

9.4 7.1 8.6 9.5 12.5 13.1 14.1 12.1 11.2

Weighted Mean 11.1 (100.0%) 1980 01

02 03 04 05 06 07 08 09 10 11 12

63 20 16 76 63 87 34 47 27 96 45 70 Sum 644

rain 9.2 4.7 10.2

6.5 6.2 7.3 6.2 7.9 7.6 13.3 16.6 8.5

Weighted Mean 8.9 (100.0%)

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TABLE 13

NARRABRI Station : 053030

Latitude: 30 20S Longitude: 149 45E Altitude: 212.4 m

Year

1 CWO

Month

r\-\W 0.

02 03 04 05 06 07 08 09 10 11 12

Precipitation (a)

-rn/ w

7 69 5 61 64 10 24 64 31 73 5 Sum 483

Type

i. a. .LIl

TU C*3) 3 . o

9.7

8.3 11.5 12.5

Weighted Mean 10.3 (63.6%) 1980 01

02 03 04 05 06 07 08 09 10 11 12

60 67 12 3 136 20 24 14 0 50 10 90 Sum 486

rain 7.9

8.5

8.0

Weighted Mean 8.1 (41.2%)

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PERTH Station : 009021

Latitude: 31 55s Longitude: 115 58E Altitude: 17.1 m

Year 1979

Month 01 02 03 04 05 06 07 08 09 10 11 12

Precipitation (a) 0

12 20 41 68 145 76 89 37 24 51 5 Sum 568

Type rain

TU (b>

9.6 5.3 4.4 3.9 4.3 5.7 6.4 6.5 3.8 5.5 5.0

Weighted Mean 5.2 (100.0%) 1980 01

02 03 04 05 06 07 08 09 10 11 12

0 14 2 77 87 135 157 108 58 36 12 14 Sum 700

11.3 9.5 5.0 5.2 5.2 4.5 4.2 6.6 4.2 4.9 5.6

Weighted Mean 5.1 (100.0%)

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TABLE 15

RYDE Station : 066062

Latitude: 33 52S Longitude: 151 12E Altitude: 92.0 m

Year 1979

Month 01 02 03 04 05 06 07 08 09 10 11 12

Precipitation (a) 115

18 192 26 115 171 27 8 25 47 67 3 Sum 814

Type rain

TU (V 4.4 5.9 8.1 10.3 5.6 3.7 10.0 18.8 18.3 13.2 16.9 6.7

Weighted Mean 7.8 (100.0%) 1980 01

02 03 04 05 06 07 08 09 10 11 12

173 75 66 12 125 48 44 14 6 32 60 81 Sum 736

rain 4.7 5.8 4.1 • 8.9 3.1 5.7 5.4 9.8 8.7 10.7 10.7 5.9

Weighted Mean 5.7 (100.0%) The precipitation figures are for Sydney Regional Office which is situated 12 km from Ryde. No precipitation figures for Ryde are available.

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TOOWOOMBA Station : 041103

Latitude: 27 35S Longitude: 151 56E Altitude: 675.0 m

Year 1979

Month Cl 02 03 04 05 06 07 08 09 10 11 12

Precipitation (&) 123

86 164 14 56 92 51 11 27 110 120 61 Sum 920

Type rain

TU (b)

3 . 9 5.7 8.0 7.0 6.3 2.8 7.3 11.2 13.9 6.6 7.1 6.8

Weighted Mean 6.4 (100.0%) 1980 01

02 03 04 05 06 07 08 09 10 11 12

95 97 39 14 117 12 67 30 3 154 55 271 Sum 954

rain 7.3 4.9 4.7 6.8 3.3 5.9 9.0 7.5 8.6 8.5 8.7 6.7

Weighted Mean 6>7 (100.0%)

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Printed by the AAEC Research Establishment

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TABLE 10 LONGREACH

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