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4.5 Critical Temperature versus Energy Gap

4.5.3 Discussion

h

Figure 4.10: Apparent energy gaps versus normalized Zeeman energy η.

the in-plane magnetic field would reduce the stability of the correlated state and thus likely results in a decrease in a band gap for charged excitations. Also, the full spin polarization of the competing CF phase could lead to a lessened screening of disorder and enhanced hopping conduction between localized states; consequently, the energy scale associated with variable-ranged or nearest-neighbor hopping would decrease. In either case, figure 4.10 strongly suggests that the gap for charged excitations does not increase with tilt angles. This is in agreement with a previous study of transport at νT = 1 in the presence of a large parallel field [42], which found that the charge gap at low d/` was independent of Zeeman energy.

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the location of the phase boundary does not influence the properties of the correlated state at low temperature. Here, an increase in Zeeman energy increasesTc.

In a first-order phase transition, the location of the phase boundary should be governed by a series of Clausius-Clapeyron relations. For example, Zou et al. [139]

did an extensive survey of the various experimental studies in which theνT = 1 phase boundary shifted in response to Zeeman energy, temperature, and density imbalance.

Assuming that the phase transition was first order, they calculated the behavior of the phase boundaries when these three parameters were tuned. They found good agreement between their model and experimental data using the approximation,

∂(∆F)

∂x =γ e2

`3. (4.5)

Here, ∆F ≡Fcorr −Funcorr is the difference between the free energy densities of the correlated and uncorrelated phases and γ was a constant that they determined by fitting their models ofFcorr andFuncorr to the experimental results. They determined that the value of γ = (1±0.1)×10−3 best fits the full set of data.

Although Zou et al. were focused on calculating (d/`)c, we can extend their anal- ysis to predict the evolution of Tc as a function of Zeeman energy. We first invoke the Clausius-Clapeyron relation

dT

dEZ = NTuncorr−ξcorr)

∂Funcorr

∂T∂F∂Tcorr (4.6)

to describe the slope of the phase boundary in T −EZ space. The numerator on the right-hand side of equation (4.6) reflects the difference in spin polarization of the two phases, with NT denoting the total electron density. The denominator is the difference in entropy of the two phases.

We will invoke a number of simplifying assumptions about the correlated and uncorrelated phases, so as to derive a mainly qualitative prediction for the behavior of the phase boundary. First, we ignore any spin-flip excitations in the correlated phase, such thatξcorr = 1 for the relevant temperatures. As suggested in the previous

estimate ξuncorr = η/ηc, where ηc is the critical Zeeman energy that is required to fully spin polarize the uncorrelated phase at a fixed, finite temperature. As seen in figure 4.7c, this term will grow with temperature and is expected to be ηc ≈0.02 in the relevant temperature range of T ≈200−300 mK. For now, we will assume that ηc is a constant whose value will be used as a fitting parameter when comparing the theoretical behavior of Tc with our observed data.

Third, we will ignore the contributions of both pseudospin waves and Chern-Simon gauge field fluctuations in the entropy term ∂Funcorr∂T∂F∂Tcorr. This is motivated by the observation of Zou et al. that such contributions are negligible compared to the noninteracting composite fermion entropy density. Finally, we will restrict ourselves to the case of η ≤ ηc; beyond η = ηc, the critical temperature should be essentially constant.

These assumptions allow us to write equation (4.6) as, dT

dEZ = 1−η/ηc

αT , (4.7)

where α = h22mCF`2k2b, mCF is the composite fermion mass, and kb is Boltzmann constant. Choosing a proper value formCF can be incredibly tricky. We must empha- size that composite fermions can appear to have different effective masses in different contexts [58]. For example, one can define a polarization mass mp based on the con- dition EF¯h2m2k2F

p = EZ; such a mass should reflect the full depth of the composite fermion Fermi sea. However, here we are interested in the thermodynamical proper- ties of the composite fermions. The massmCF denotes the composite fermion mass if we could treat the system as comprising of nearly free fermions with the same entropy per particle as the composite fermion system. Consequently, mCF should provide a measure of the density of states in the vicinity of the Fermi energy. A theoretical estimate [50] for this type of mass arrives at the value mCF ≈ 0.079 mep

B[T],

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whereme is the electron mass in vacuum.3 However, the true value of mCF in a given sample is expected to be strongly affected by the finite thickness of the quantum well, disorder, and Landau level mixing [133, 88, 89, 83]. Because such conditions should vary from sample to sample, there should not be a universal value for mCF. For this reason, we will use mCF as another fitting parameter that can be varied to best fit our data.

Simple algebraic manipulation and then integration of the ODE shown in equation (4.7) lead to

T2 = 2EC

α η− EC

αηcη2+C0, (4.8)

whereC0 is an arbitrary constant. Thus, one expects a plot ofTc2 versusη to follow a parabolic curve whose peak coincides with the full spin polarization of the CF phase.

The square of the observed critical temperature as a function of normalized Zee- man energy is shown in figure 4.11. A parabolic fit to the data givesTc2 =C0+C1η+ C2η2, with C0 = (−0.00777±0.0044), C1 = (15.92±0.65), and C3 = (−329±22).

From these fitting parameters, one obtains ηc = 0.024 and mCF = 1.36mep

B[T].

These values are in partial agreement with the expected ηc ≈ 0.02 (as expected for this range of temperatures in figure 4.7c) andmCF = 0.2mep

B[T], which is the CF mass as used by Zou et al. in reference [139]. This value for the composite fermion mass originates from the measurement of activation gaps in the vicinity of ν = 1/2 by Duet al. [15, 17]. If one instead employs these values for ηc andmCF, one arrives at the red dotted line in figure 4.11. Note that in the predictedTc2 versusη curve, we also choose to use a different value of the arbitrary constant C0 so as to match with the observed Tc2 value at zero tilt angle.

It should be clear from figure 4.11 that the observed critical temperature grows much more slowly with Zeeman energy than expected. There are several possible ex- planation for this discrepancy. One possibility is that our assumption that the entropy of the composite fermion phase scales linearly with temperature is an oversimplifica-

3Although the effective masses of composite fermions are often given in terms ofme, this formal- ism is somewhat misleading because their properties should in principle be completely unrelated to the bare electron mass [58].

h

Figure 4.11: Expected and observed Tc2 versus η at d/`= 1.59. The solid black line is a parabolic fit to the observed data points.

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tion. While that behavior is reasonable for noninteracting fermions, the entropy of a composite fermion system at ν = 12 will include contributions from gauge fluctua- tions that scale either asT2/3 for the case of short-range interactions or asT lnT for long-range Coulomb interactions (for example, see references [50] and [139]). Another possibility for the discrepancy between the theoretical curve and experimental curve is that our particular definition of Tc does not track precisely with the true location of the phase boundary. Also, the value of mCF that Zou et al. uses might not be appropriate for our particular double quantum-well system in the presence of a large parallel magnetic field. As mentioned earlier, mCF can be sensitive to the effective thickness of the quantum well and disorder, both of which might be modified by the in-plane field. Finally, we note the possibility that the correlated phase is not fully spin polarized at the phase boundary.