WAVEGUIDE QUANTUM ELECTRODYNAMICS
2.3 Waveguide QED in a dispersive photonic channel
While the original concept of waveguide QED revolved around coupling quantum emitters to a waveguide inside a transmission band, a new paradigm to induce long-range photon-mediated interactions between quantum emitters inside a pho- tonic bandgap was proposed in Ref. [125]. In this scheme, photonic structures are engineered to host a bandgap where the propagation of photons are prohibited. Tun- ing the emitters’ frequencies inside the bandgap, the emitters cannot radiate to the waveguide channel while the coherent interaction between distant emitters are still allowed by means of exchange of virtual photons. Compared to the case when the emitters are tuned inside the transmission band discussed in Sec. 2.2, the bandgap regime offers a practical direction to achieve strong and long-range coupling be- tween emitters without suffering from significant dissipation to the photonic band.
In this section, I introduce the basic concepts of this direction to achieve a scalable quantum many-body system with long-range connectivity.
Emitter-photon bound states
When the transition frequency of a quantum emitter is tuned inside a photonic bandgap of an electromagnetic structure, the spontaneous emission of the emitter is forbidden due to the absence of resonant photonic modes to absorb the emitted
d
a
ξb
−π/d 0 π/d k ω
ωc
ω0
ωb BG
Figure 2.7: Emitter-photon bound state. a, Illustration of a quantum emitter (green circle) coupled to a 1D dispersive waveguide channel (gray) represented as a periodic electromagnetic structure with lattice constant 𝑑. The emitter’s frequency is tuned inside the bandgap of the waveguide, inducing a emitter-photon bound state exponentially localized at a length scale𝜉, shaded in blue.b,An example of photonic bandstructure of a dispersive waveguide. The transmission band (bandgap) is shaded in red (gray). Tuning the bare transition frequency𝜔0of the emitter (green arrow) below the frequency𝜔𝑐of band-edge, the emitter-photon bound state exists at a frequency𝜔𝑏lower than that of the emitter (blue arrow).
photons. Instead, the emitted photon is scattered back to the original emitter, resulting in a coupled eigenstate of photonic modes of the electromagnetic structure and the emitter. This is known as theemitter-photon bound state3, first predicted by Sajeev John and Jian Wang in 1990 [126] in the context of Anderson localization of light [127]. In the emitter-photon bound state, the emitter is dressed with a photonic tail exponentially localized with respect to the emitter, gaining a spatial extent. This length scale of the emitter-photon bound state can be adjusted by controlling the detuning of the emitter from the edge of the photonic band.
The Hamiltonian of a quantum emitter coupled to such 1D photonic structure, a dispersive waveguide (an example illustrated in Fig. 2.7), can be written as
ˆ
𝐻 = ℏ𝜔0|𝑒ih𝑒| +Õ
𝑘
ℏ𝜔𝑘𝑎ˆ†
𝑘𝑎ˆ𝑘 +Õ
𝑘
ℏ
𝑔𝑘𝑎ˆ†
𝑘|𝑔ih𝑒| +𝑔∗
𝑘𝑎ˆ𝑘|𝑒ih𝑔|
, (2.14) where 𝜔0 is the transition frequency of the emitter, ˆ𝑎𝑘 ( ˆ𝑎†
𝑘) is the annihilation (creation) operator of photonic mode at wavevector𝑘 satisfying the canonical com- mutation relation[𝑎ˆ𝑘,𝑎ˆ†
𝑘0] =𝛿𝑘 , 𝑘0, and𝑔𝑘is the momentum-space coupling between the emitter and the waveguide photons. Here, |𝑔i and |𝑒idenote the ground state and the excited state of the emitter, respectively. Limiting our analysis to the single-
3Also known as the atom (qubit)-photon bound state if an atom (a qubit) plays the role of a two- level emitter.
excitation manifold, we look for a emitter-photon bound state of the following form
|𝜙𝑏i=cos𝜃|{0}i|𝑒i +sin𝜃 Õ
𝑘
𝑐𝑘𝑎ˆ†
𝑘|{0}i|𝑔i (2.15) that satisfies the time-independent Schrödinger equation ˆ𝐻|𝜙𝑏i = ℏ𝜔𝑏|𝜙𝑏i. Here,
|{0}i represents the vacuum state of photon modes and the coefficients 𝑐𝑘 are normalized byÍ
𝑘 |𝑐𝑘|2=1. Writing out the algebraically independent terms in the equation we get
𝜔0cos𝜃+ Õ
𝑘
𝑔∗
𝑘𝑐𝑘
!
sin𝜃 =𝜔𝑏cos𝜃 (2.16a) 𝜔𝑘𝑐𝑘sin𝜃+𝑔𝑘cos𝜃 =𝜔𝑏𝑐𝑘sin𝜃 (2.16b) From equating the coefficients in Eq. (2.16b), we obtain the probability amplitudes at wavevector 𝑘to be
𝑐𝑘 = 𝑔𝑘 (𝜔𝑏−𝜔𝑘)tan𝜃
. (2.17)
Substituting the Eq. (2.17) into Eq. (2.16a), we get a transcendental equation for evaluating the energy of the emitter-photon bound state
𝜔𝑏=𝜔0+Õ
𝑘
|𝑔𝑘|2 𝜔𝑏−𝜔𝑘
(2.18a) subjected to the normalization condition
tan2𝜃 =Õ
𝑘
|𝑔𝑘|2
(𝜔𝑏−𝜔𝑘)2. (2.18b)
For a generic 1D waveguide with a quadratic dispersion relation, a simple analytical relation to describe the emitter-photon bound state can be derived. We specifically consider the dispersion relation of the form
𝜔𝑘 =𝜔𝑐+𝛼(𝑘− 𝑘0)2, (2.19) where𝜔𝑐 is the frequency of the band-edge,𝛼 > 0 is the curvature of the photonic band, and𝑘0is the wavevector at which the band-edge occurs.
Assuming that the coupling of emitter and the waveguide locally occurs at position 𝑥 = 𝑥0 with the strength 𝑔, the emitter-photon interaction Hamiltonian takes the form ˆ𝐻int = 𝑔(𝑎ˆ†
x0|𝑔ih𝑒| +𝑎ˆx
0|𝑒ih𝑔|) in terms of real-space annihilation operator ˆ
𝑎𝑥
0 = √1
𝑁
Í
𝑘𝑒𝑖 𝑘 𝑥0𝑎ˆ𝑘 where 𝑁 is the number of modes inside the band. This is
translated into the last term in Eq. (2.14) with momentum-space coupling given by 𝑔𝑘 =𝑔 𝑒−𝑖 𝑘 𝑥0/√
𝑁. In this case, the Eqs. (2.18a)-(2.18b) are simplified into4 𝜔0−𝜔𝑏 = 𝑔2𝑑
2p
𝛼(𝜔𝑐−𝜔𝑏) (2.20a)
and
tan2𝜃 = 𝑔2𝑑 4p
𝛼(𝜔𝑐−𝜔𝑏)3
= 𝜔0−𝜔𝑏
2(𝜔𝑐−𝜔𝑏). (2.20b) Here,𝑑is the shortest length scale (lattice constant) of the waveguide that determines the first Brillouin zone. It can be seen from Eq. (2.20a) that the emitter-photon bound state inside the bandgap (𝜔𝑏 < 𝜔𝑐) has a frequency lower than the bare emitter frequency (𝜔𝑏 < 𝜔0) due to the negative Lamb shift from hybridization with photonic modes at higher frequencies. Also, combining Eqs. (2.20a)-(2.20b), it can be shown that the photonic component of the bound state becomes
sin2𝜃 =
1+4√ 𝛼 𝑔2𝑑
(𝜔𝑐−𝜔𝑏)3/2 −1
. (2.21)
This means that the emitter-photon bound state becomes more photon (emitter)-like as the frequency get closer to (farther from) the band-edge frequency𝜔𝑐.
One can also evaluate the real-space coefficients𝑐𝑥 = √1
𝑁
Í
𝑘𝑒𝑖 𝑘 𝑥𝑐𝑘 of photonic part of the wavefunction|𝜙𝑏iusing Eq. (2.17)5:
𝑐𝑥 =− 𝑔 𝑑 p2𝛼(𝜔0−𝜔𝑏)
𝑒𝑖 𝑘0(𝑥−𝑥0)𝑒−|𝑥−𝑥0|/𝜉 (2.22) where
𝜉 =
r 𝛼 𝜔𝑐−𝜔𝑏
(2.23)
4In the derivation, the summationÍ
𝑘 over the first Brillouin zone was replaced with the integral
𝑑 2𝜋
∫
𝑑 𝑘 in the thermodynamic limit (𝑁→ ∞) whose upper and lower limits are extended from±𝜋 to±∞assuming that the integration performed at high|𝑘|values are negligible. Also, the integral identities
∫ d𝑥 𝑎2+𝑥2
= 1
𝑎tan−1𝑥 𝑎
,
∫ d𝑥 𝑎2+𝑥2
2
= 1 2𝑎3
𝑎𝑥 𝑎2+𝑥2
+ 1
2𝑎3tan−1𝑥 𝑎
are employed.
5Here, the integral identity
∫ ∞
−∞
d𝑥 𝑒𝑖 𝑎 𝑥
𝑥2+1 =𝜋 𝑒− |𝑎| is used.
−π/d 0 π/d k ω
ωc
BG (i)
(ii)
Figure 2.8: Waveguide-mediated interactions between emitter-photon bound states.
When two quantum emitters are tuned inside the bandgap, the spatial overlap of correspond- ing emitter-photon bound states induces emitter-emitter interaction. The range of interaction depends on the localization length𝜉which is long when the emitters are tuned close to the band-edge frequency𝜔𝑐 (i, green arrow), while the interaction is short-ranged deep inside the bandgap (ii, blue arrow).
is the localization length. Equations (2.22)-(2.23) directly shows a few important properties of the photonic component of the bound state. First, the magnitude of 𝑐𝑥 exponentially decays at a length scale 𝜉 with respect to the location 𝑥 = 𝑥0 of the emitter. The localization length 𝜉 characterizes the effective spatial extent of the emitter-photon bound state. Second, the probability amplitude 𝑐𝑥 collects an additional factor𝑒𝑖 𝑘0(𝑥−𝑥0) associated with propagation with wavevector 𝑘 = 𝑘0 of the band-edge. Also, the localization length is inversely proportional to the detuning of bound state from the band-edge, i.e.,𝜉 ∝ (𝜔𝑐−𝜔𝑏)−1/2, diverging as𝜔𝑏 → 𝜔𝑐. This means that the spatial extent of the emitter-photon bound state can take a wide range of values depending on the frequency tuning of the emitter inside the bandgap.
Waveguide-mediated interactions between emitter-photon bound states
The spatially extended nature of the emitter-photon bound state has been viewed as a method to induce effective interactions between emitters not long since the first theoretical investigation of emitter-photon bound states [128, 129]. When two resonant emitters are tuned inside the bandgap of a common photonic structure, it was shown that the photonic band off-resonantly mediates exchange interaction between the emitters in a way similar to how each emitter is dressed by photonic modes to form the emitter-bound state (self-interaction). Such interaction takes a special form that falls off exponentially with the distance between the emitters, whose length scale𝜉 can be tuned by adjusting the frequency of the emitters inside
the bandgap (see Fig. 2.8).
The Hamiltonian of two quantum emitters (labeled by𝑗 =1,2) coupled to a common 1D dispersive waveguide is given by
ˆ 𝐻 =Õ
𝑗
ℏ𝜔(𝑗)
0 |𝑒ih𝑒|𝑗+Õ
𝑘
ℏ𝜔𝑘𝑎ˆ†
𝑘𝑎ˆ𝑘 +Õ
𝑗 , 𝑘
ℏh 𝑔(𝑗)
𝑘 𝑎ˆ†
𝑘|𝑔ih𝑒|𝑗 +𝑔(𝑗)
𝑘
∗𝑎ˆ𝑘|𝑒ih𝑔|𝑗
i , (2.24) where𝜔(𝑗)
0 is the frequency of the emitter 𝑗, ˆ𝑎𝑘 ( ˆ𝑎†
𝑘) is the annihilation (creation) operator of photonic mode at wavevector 𝑘 satisfying the canonical commutation relation [𝑎ˆ𝑘,𝑎ˆ†
𝑘0] = 𝛿𝑘 , 𝑘0, and 𝑔(𝑗)
𝑘 is the momentum-space coupling between the emitter 𝑗 and the waveguide. Here, |𝑔i𝑗 and |𝑒i𝑗 denote the ground state and the excited state of the emitter 𝑗, respectively.
Again, we look for a emitter-photon bound state in the single-excitation manifold of the following form
|𝜙𝑏i=cos𝜃|{0}i h
𝑐𝑞(1)|𝑒i1|𝑔i2+𝑐𝑞(2)|𝑔i1|𝑒i2i +sin𝜃
Õ
𝑘
𝑐𝑘𝑎ˆ†
𝑘|{0}i|𝑔i1|𝑔i2 (2.25) that satisfies the time-independent Schrödinger equation ˆ𝐻|𝜙𝑏i = ℏ𝜔𝑏|𝜙𝑏i. Here,
|{0}i represents the vacuum state of photon modes and the coefficients 𝑐𝑘 are normalized byÍ
𝑘|𝑐𝑘|2=1 and𝑐𝑞 byÍ
𝑗 |𝑐(
𝑗)
𝑞 |2=1. Writing out the algebraically independent terms in the equation we get
𝜔(
𝑗) 0 𝑐(
𝑗)
𝑞 cos𝜃+ Õ
𝑘
𝑔(
𝑗) 𝑘
∗
𝑐𝑘
!
sin𝜃 =𝜔𝑏𝑐(
𝑗)
𝑞 cos𝜃 , (2.26a) Õ
𝑗
𝑔(𝑗)
𝑘 𝑐(𝑞𝑗)
!
cos𝜃+𝜔𝑘𝑐𝑘sin𝜃 =𝜔𝑏𝑐𝑘sin𝜃 . (2.26b) Equation (2.26b) can be simplified into an expression for coefficients𝑐𝑘of photonic modes:
𝑐𝑘 = Í
𝑗𝑔(
𝑗) 𝑘
𝑐(
𝑗) 𝑞
(𝜔𝑏−𝜔𝑘)tan𝜃
. (2.27)
Substituting Eq. (2.27) into Eq. (2.26a), we obtain an eigenequation for probability amplitudes𝑐(
𝑗)
𝑞 of quantum emitters given by 𝜔𝑏
𝑐(𝑞1) 𝑐(𝑞2)
!
= 𝜔(1)
0 +𝐽11 𝐽12 𝐽21 𝜔(2)
0 +𝐽22
! 𝑐(𝑞1) 𝑐(𝑞2)
!
, (2.28)
where
𝐽𝑖 𝑗 =Õ
𝑘
𝑔(𝑖)
𝑘
∗
𝑔(
𝑗) 𝑘
𝜔𝑏−𝜔𝑘
. (2.29)
The matrix 𝐽𝑖 𝑗 is Hermitian and represents the effective interaction between the emitters mediated by photons of the transmission band. The diagonal terms (𝑖= 𝑗) correspond to self-interaction of a quantum emitter with itself, also known as the Lamb shift identical to Eq. (2.18a).
Considering again a 1D waveguide with a quadratic dispersion relation described in Eq. (2.19) where each emitter 𝑗 is coupled at position𝑥 = 𝑥𝑗 of the waveguide (resulting in momentum-space coupling𝑔(𝑗)
𝑘 =𝑔 𝑒−𝑖 𝑘 𝑥𝑗/√
𝑁), we can readily evaluate the sum over 𝑘 in the thermodynamic limit. Following procedures similar to the derivation of Eq. (2.22), Equation (2.29) reduces to
𝐽𝑖 𝑗 =− 𝑔2𝑑 2p
𝛼(𝜔𝑐−𝜔𝑏)
𝑒𝑖 𝑘0(𝑥𝑖−𝑥𝑗)𝑒−|𝑥𝑖−𝑥𝑗|/𝜉, (2.30) where 𝜉 is the localization length defined in (2.23). It can be easily seen that the interaction between emitters mediated by the dispersive waveguide in Eq. (2.30) follows the spatial shape of emitter-photon bound state in Eq. (2.22), collecting a phase factor 𝑒𝑖 𝑘0Δ𝑥 and an attenuation factor 𝑒−|Δ𝑥|/𝜉 associated with suppressed propagation of a photon inside the bandgap along the displacement Δ𝑥 = 𝑥𝑖 −𝑥𝑗 between the emitters.